FM synthesis telling a story about game development. That's already incredible. Soft de Hard na Monogatari by System Sacom is a visual novel about the chaos of making games, and the X68000 soundtrack nails every mood shift with sharp FM tones.
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Nichijou has this light, everyday feel that lulls you in, but then Mondai Hassei hits and the tension ramps up hard. The RPG no Theme track is a fun meta moment where you hear the game-within-a-game's music. Programmer Ondo at the end is genuinely charming.
Three unused tracks hiding in there too. If you're a developer or anyone who's ever crunched on a deadline, this soundtrack is going to hit different.