If you already own the Jin no Shou soundtrack, this is basically the expanded director's cut. Tokyo Majin Gakuen Sougakushou Ten no Shou by Takashi Nitta shares about 70% of its tracklist with the previous album since it was a PS1-to-PS2 port, but the new additions are worth hearing.
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"Springtime Guardian" and "Falling Cherry Blossoms" bring fresh melodic ideas to the same Taishou-era folk palette. "Flower Garden March" and "Hymn to the Sky" add brightness the first album didn't quite reach. The synth quality is basically unchanged though.
Worth it for the exclusive tracks if you're already a fan of Nitta's supernatural school sound, but start with Jin no Shou if you're picking one.