"Engage the Enemy" might be one of the most emotionally devastating battle themes ever written. The Xenoblade Chronicles Trinity Box collects Yoko Shimomura, ACE+, Manami Kiyota, and Yasunori Mitsuda's work in Definitive Edition quality, and it sounds incredible.
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"Colony 9" has that warm daytime energy that immediately feels like home, and then the night version strips it down to something gentle and reflective. "Gaur Plain" lives rent-free in every Xenoblade fan's head for a reason.
The way the day/night cycle changes the entire emotional texture of each area... honestly unmatched. If you played the original on Wii and never revisited, the reorchestrated versions alone are worth coming back for.