Akira Yamaoka literally wrote a rock album disguised as a PS2 horror soundtrack and nobody talks about it enough. Silent Hill 3's limited edition pulls the vocal tracks into focus, and You're Not Here goes so hard it ended up on DDR.
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Breeze - in Monochrome Night has this fragile acoustic thing happening that makes you forget you were just running from monsters five minutes ago. Letter - from the Lost Days is Mary Elizabeth McGlynn at her most gut-punch honest, the kind of vocal performance that sits in your chest.
That contrast between soft and aggressive. If you ever wanted proof horror games produce the best singers, start here.