This soundtrack hits darker than any other Zelda and it works so well. Twilight Princess HD on Wii U brought Toru Minegishi and company's score into cleaner fidelity and you can really hear how much weight every piece carries now.
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Midna's Theme alone is worth it, this delicate piano line that keeps folding in on itself until it just aches. Then you've got Hyrule Field Main Theme doing this slow orchestral build that makes riding Epona feel genuinely epic.
The Twilight battle tracks go hard too, all tension and these anxious string runs that the normal battle music doesn't touch. Something about Light Spirit's Elegy that just stays with you. If you only know Wind Waker Zelda, this is the one that'll change your mind about what these soundtracks can do.